全文获取类型
收费全文 | 2799篇 |
免费 | 81篇 |
国内免费 | 24篇 |
专业分类
安全科学 | 123篇 |
废物处理 | 110篇 |
环保管理 | 843篇 |
综合类 | 282篇 |
基础理论 | 677篇 |
环境理论 | 1篇 |
污染及防治 | 590篇 |
评价与监测 | 161篇 |
社会与环境 | 79篇 |
灾害及防治 | 38篇 |
出版年
2023年 | 16篇 |
2022年 | 20篇 |
2021年 | 32篇 |
2020年 | 22篇 |
2019年 | 38篇 |
2018年 | 52篇 |
2017年 | 53篇 |
2016年 | 68篇 |
2015年 | 56篇 |
2014年 | 60篇 |
2013年 | 307篇 |
2012年 | 112篇 |
2011年 | 140篇 |
2010年 | 112篇 |
2009年 | 123篇 |
2008年 | 161篇 |
2007年 | 145篇 |
2006年 | 129篇 |
2005年 | 98篇 |
2004年 | 80篇 |
2003年 | 98篇 |
2002年 | 87篇 |
2001年 | 58篇 |
2000年 | 50篇 |
1999年 | 26篇 |
1998年 | 45篇 |
1997年 | 30篇 |
1996年 | 39篇 |
1995年 | 48篇 |
1994年 | 34篇 |
1993年 | 46篇 |
1992年 | 38篇 |
1991年 | 19篇 |
1990年 | 23篇 |
1989年 | 18篇 |
1988年 | 24篇 |
1987年 | 15篇 |
1986年 | 19篇 |
1985年 | 28篇 |
1984年 | 23篇 |
1983年 | 25篇 |
1982年 | 34篇 |
1981年 | 37篇 |
1980年 | 34篇 |
1979年 | 22篇 |
1978年 | 24篇 |
1977年 | 11篇 |
1976年 | 9篇 |
1974年 | 8篇 |
1972年 | 10篇 |
排序方式: 共有2904条查询结果,搜索用时 218 毫秒
91.
Thomas J. Kulle Larry R. Sauder J. Richard Hebel Donald J. Green Marie D. Chatham 《Journal of the Air & Waste Management Association (1995)》2013,63(8):919-924
Industrial, commercial, and domestic levels of formaldehyde exposure range from <0.1 to >5.0 ppm. Irritation of the eyes and upper respiratory tract predominate, and bronchoconstriction is described in case reports. However, pulmonary function and irritant symptoms together have not been assessed over a range of HCHO concentrations in a controlled environment. We investigated dose response in both symptoms and pulmonary function associated with 3-h exposures to 0.0-3.0 ppm HCHO in a controlled environmental chamber. Ten subjects were randomly exposed to 0.0, 0.5, 1.0, and 2.0 ppm HCHO at rest plus 2.0 ppm HCHO with exercise and nine additional subjects were randomly exposed to 0.0,1.0,2.0, and 3.0 ppm HCHO at rest plus 2.0 ppm HCHO with exercise. Significant dose-response relationships in odor and eye irritation were observed (p < 0.05). Nasal flow resistance was increased at 3.0 ppm (p < 0.01), but not at 2.0 ppm HCHO. There were no significant decrements in pulmonary function (FVC, FEV1, FEF25-75%, SGaw) or increases in bronchial reactivity to methacholine (log PD35SGaw) with exposure to 0.5-3.0 ppm HCHO at rest or to 2.0 ppm HCHO with exercise. 相似文献
92.
Sharon Sjostrom Tim Ebner Trevor Ley Richard Slye Carl Richardson Tom Machalek 《Journal of the Air & Waste Management Association (1995)》2013,63(8):902-911
Abstract Sorbent injection for Hg control is one of the most promising technologies for reducing Hg emissions from power-generation facilities, particularly units that do not require wet scrubbers for SO2 control. Since 1992, EPRI has been assessing the performance of Hg sorbents in pilot-scale systems installed at full-scale facilities. The initial tests were conducted on a 5000-acfm (142-m3/min) pilot baghouse. Screening potential sorbents at this scale required substantial resources for installation and operation and did not provide an opportunity to characterize sor-bents over a wide temperature range. Data collected in the laboratory and in field tests indicate that sorbents are affected by flue gas composition and temperature. Tests carried out in actual flue gas at a number of power plants also have shown that sorbent performance can be site-specific. In addition, data collected at a field site often are different from data collected in the laboratory, with simulated flue gas mixed to match the major components in the site’s gas. To effectively estimate the costs of Hg sorbent systems at different plants, a measure of sorbent performance in the respective flue gases must be obtained. However, injection testing at multiple facilities with large pilot systems is not practical. Over the past five years, fixed-bed characterization testing, modeling studies, and bench-scale injection testing have been undertaken to develop a low-cost technique to characterize sorbent performance in actual flue gas and subsequently to project normalized costs for Hg removal prior to full-scale demonstration. This article describes the techniques used and summarizes field-testing results from two plants burning Powder River Basin (PRB) coal for commercial activated carbon and several other sorbent types. Full-scale projections based on the results and data collected on larger-scale systems also are included. 相似文献
93.
94.
Carl Folke Stephen Polasky Johan Rockstrm Victor Galaz Frances Westley Michle Lamont Marten Scheffer Henrik
sterblom Stephen R. Carpenter F. Stuart Chapin III Karen C. Seto Elke U. Weber Beatrice I. Crona Gretchen C. Daily Partha Dasgupta Owen Gaffney Line J. Gordon Holger Hoff Simon A. Levin Jane Lubchenco Will Steffen Brian H. Walker 《Ambio》2021,50(4):834
The COVID-19 pandemic has exposed an interconnected and tightly coupled globalized world in rapid change. This article sets the scientific stage for understanding and responding to such change for global sustainability and resilient societies. We provide a systemic overview of the current situation where people and nature are dynamically intertwined and embedded in the biosphere, placing shocks and extreme events as part of this dynamic; humanity has become the major force in shaping the future of the Earth system as a whole; and the scale and pace of the human dimension have caused climate change, rapid loss of biodiversity, growing inequalities, and loss of resilience to deal with uncertainty and surprise. Taken together, human actions are challenging the biosphere foundation for a prosperous development of civilizations. The Anthropocene reality—of rising system-wide turbulence—calls for transformative change towards sustainable futures. Emerging technologies, social innovations, broader shifts in cultural repertoires, as well as a diverse portfolio of active stewardship of human actions in support of a resilient biosphere are highlighted as essential parts of such transformations. 相似文献
95.
Shahid Parvez Glenn E. Rice Linda K. Teuschler Jane Ellen Simmons Thomas F. Speth Susan D. Richardson Richard J. Miltner E. Sidney Hunter III Jonathan G. Pressman Lillian F. Strader Gary R. Klinefelter Jerome M. Goldman Michael G. Narotsky 《环境科学学报(英文版)》2017,29(8):311-321
A method based on regression modeling was developed to discern the contribution of component chemicals to the toxicity of highly complex, environmentally realistic mixtures of disinfection byproducts(DBPs). Chemical disinfection of drinking water forms DBP mixtures.Because of concerns about possible reproductive and developmental toxicity, a whole mixture(WM) of DBPs produced by chlorination of a water concentrate was administered as drinking water to Sprague–Dawley(S–D) rats in a multigenerational study. Age of puberty acquisition,i.e., preputial separation(PPS) and vaginal opening(VO), was examined in male and female offspring, respectively. When compared to controls, a slight, but statistically significant delay in puberty acquisition was observed in females but not in males. WM-induced differences in the age at puberty acquisition were compared to those reported in S–D rats administered either a defined mixture(DM) of nine regulated DBPs or individual DBPs. Regression models were developed using individual animal data on age at PPS or VO from the DM study. Puberty acquisition data reported in the WM and individual DBP studies were then compared with the DM models. The delay in puberty acquisition observed in the WM-treated female rats could not be distinguished from delays predicted by the DM regression model, suggesting that the nine regulated DBPs in the DM might account for much of the delay observed in the WM. This method is applicable to mixtures of other types of chemicals and other endpoints. 相似文献
96.
Chandra Nath Shiv G. Kapoor Richard E. DeVor Anil K. Srivastava Jon Iverson 《Journal of Manufacturing Processes》2012,14(4):452-459
Tool life has been a vital issue in machining titanium alloys. Recently, an atomization-based cutting fluid (ACF) application has been found to be an effective approach for cooling and lubrication in micromachining operations. In this study, an ACF spray system is developed for macro-scale turning of Ti–6Al–4V. The spray system is designed to minimize interaction between the fluid droplets, and the gas nozzle to control the divergence of the fluid droplets. Experiments are conducted to study the effect of five specific ACF spray parameters including fluid flow rate, spray distance, impingement angle, and type and pressure level of the droplet carrier gas on cutting forces, tool life, and chip characteristics. It has been observed that the combination of lower pressure (150 psi) air-mixed CO2 with a higher flow rate (20 ml/min) and a larger spray distance (35 mm) produces a significantly longer tool life and broken chips. The results also reveal that the ACF spray system can extend tool life up to 40–50% over flood cooling. 相似文献
97.
Modeling and interpretation of fiber orientation-based failure mechanisms in machining of carbon fiber-reinforced polymer composites 总被引:1,自引:0,他引:1
Kevin A. Calzada Shiv G. Kapoor Richard E. DeVor Johnson Samuel Anil K. Srivastava 《Journal of Manufacturing Processes》2012,14(2):141-149
The development and implementation of a microstructure-based finite element model for the machining of carbon fiber-reinforced polymer composites is presented. A new approach to interfacial modeling is introduced where the material interface is modeled using continuum elements, allowing failure to take place in either tension or compression. The model is capable of describing the fiber failure mode occurring throughout the chip formation process. Characteristic fiber length in the chips, and machining forces for microstructures with fibers orientated at 0°, 45°, 90°, and 135° are examined. For model validation purposes, the model-based machining performance predictions are compared to the machining responses from a set of orthogonal machining experiments. A parametric study is presented that identifies a robust tool geometry, which minimizes the effects of fiber orientation and size on the machining forces. 相似文献
98.
The double trade-off between adaptation and mitigation for sea level rise: an application of FUND 总被引:6,自引:2,他引:4
Richard S. J. Tol 《Mitigation and Adaptation Strategies for Global Change》2007,12(5):741-753
This paper studies the effects of adaptation and mitigation on the impacts of sea level rise. Without adaptation, the impact
of sea level rise would be substantial, almost wiping out entire countries by 2100, although the globally aggregate effect
is much smaller. Adaptation would reduce potential impacts by a factor 10–100. Adaptation would come at a minor cost compared
to the damage avoided. As adaptation depends on socio-economic status, the rank order of most vulnerable countries is different
than the rank order of most exposed countries. Because the momentum of sea level rise is so large, mitigation can reduce impacts
only to a limited extent. Stabilising carbon dioxide concentrations at 550 ppm would cut impacts in 2100 by about 10%. However,
the costs of emission reduction lower the avoided impacts by up to 25% (average 10%). This is partly due to the reduced availability
of resources for adaptation, and partly due to the increased sensitivity to wetland loss by adaptation.
相似文献
Richard S. J. TolEmail: |
99.
Lu Y Beeman RW Campbell JF Park Y Aikins MJ Mori K Akasaka K Tamogami S Phillips TW 《Die Naturwissenschaften》2011,98(9):755-761
We report that the abdominal epidermis and associated tissues are the predominant sources of male-produced pheromones in the
red flour beetle, Tribolium castaneum and, for the first time, describe the stereoisomeric composition of the natural blend of isomers of the aggregation pheromone
4,8-dimethyldecanal (DMD) in this important pest species. Quantitative analyses via gas chromatography–mass spectrometry showed
that the average amount of DMD released daily by single feeding males of T. castaneum was 878 ± 72 ng (SE). Analysis of different body parts identified the abdominal epidermis as the major source of aggregation
pheromone; the thorax was a minor source, while no DMD was detectable in the head. No internal organs or obvious male-specific
glands were associated with pheromone deposition. Complete separation of all four stereoisomers of DMD was achieved following
oxidation to the corresponding acid, derivatization with (1R, 2R)- and (1S, 2S)-2-(anthracene-2,3-dicarboximido)cyclohexanol to diastereomeric esters, and their separation on reversed-phase high-performance
liquid chromatography at −54°C. Analysis of the hexane eluate from Porapak-Q-collected volatiles from feeding males revealed
the presence of all four isomers (4R,8R)/(4R,8S)/(4S,8R)/(4S,8S) at a ratio of approximately 4:4:1:1. A walking orientation bioassay in a wind tunnel with various blends of the four synthetic
isomers further indicated that the attractive potency of the reconstituted natural blend of 4:4:1:1 was equivalent to that
of the natural pheromone and greater than that of the 1:1 blend of (4R,8R)/(4R,8S) used in commercial lures. 相似文献
100.
Leona Bohdalkova Martin Novak Frantisek Buzek Jakub Kreisinger Richard Bindler Katerina Pazderu Petra Pacherova 《Mitigation and Adaptation Strategies for Global Change》2014,19(7):997-1010
There are fears that global warming will lead to degradation of peatlands, higher emissions of greenhouse gases from peat, and accelerated warming. Anaerobic decomposition of organic soils produces methane (CH4), a potent greenhouse gas. Two peat bogs differing in mean annual temperature, Velke Darko (VD, Czech Republic, 7.2 °C), and Stor Åmyran (SA, Sweden, 4.0 °C), were selected for a comparative study of how organic soils in different climatic zones will respond to warmer and drier conditions. Twenty peat cores from each bog were incubated in growth chambers. Under present-day summer conditions, VD produced 14 times more CH4 than SA. Two different warming scenarios were used. Peat-core replicates were kept at temperatures of 11 versus 16 °C, and 11 versus 22 °C. From 11 to 16 °C, the CH4 production slightly decreased at SA, and slightly increased at VD. From 11 to 22 °C, the CH4 production increased 9 times at SA, but slightly decreased at VD. After an 8-month incubation, peat cores under drying conditions (water table at ?14 cm) were compared to samples with original water table (?2 cm). Drying conditions led to a steeper reduction in CH4 production at VD, compared to SA. The CH4 production decreased more than 100 times at VD. Then, the combined effect of simultaneous warming and drying at 11 and 22 °C was studied. We did not find any significant effect of interactions between increasing temperature and decreasing water table level. Overall, the warmer site VD responded more strongly to the simulated climate change than the colder site SA. 相似文献